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Creators/Authors contains: "Roberts, Trevor"

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  1. Free, publicly-accessible full text available December 1, 2025
  2. This dataset contains four raster maps of shrub community structure at the Jornada Basin LTER site in southern New Mexico U.S.A. These shrub structure estimates were created by combining an existing categorical shrub map (Ji et al. 2019) with USGS LiDAR shrub height estimates from 2019. The resulting raster dataset includes four bands of spatially aligned shrub volume, cover, height, and density estimates at one hectare resolution. Data are also included in tabular format, extracted from the 1 hectare grid upon which estimates were created. These shrub structure estimates are intended to facilitate analyses of habitat structure and community dynamics within the northern Chihuahuan Desert. 
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  3. Quantum dot (QD) solids are promising optoelectronic materials; further advancing their device functionality requires understanding their energy transport mechanisms. The commonly invoked near-field Förster resonance energy transfer (FRET) theory often underestimates the exciton hopping rate in QD solids, yet no consensus exists on the underlying cause. In response, we use time-resolved ultrafast stimulated emission depletion (STED) microscopy, an ultrafast transformation of STED to spatiotemporally resolve exciton diffusion in tellurium-doped cadmium selenide–core/cadmium sulfide–shell QD superlattices. We measure the concomitant time-resolved exciton energy decay due to excitons sampling a heterogeneous energetic landscape within the superlattice. The heterogeneity is quantified by single-particle emission spectroscopy. This powerful multimodal set of observables provides sufficient constraints on a kinetic Monte Carlo simulation of exciton transport to elucidate a composite transport mechanism that includes both near-field FRET and previously neglected far-field emission/reabsorption contributions. Uncovering this mechanism offers a much-needed unified framework in which to characterize transport in QD solids and additional principles for device design. 
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